roughly speaking, ATI currently has the better hardware (faster, less power draw) and is more Open Source friendly (offering specs, developing drivers), but when you compare the binary drivers nvidia's are still better.
However, the question is: what are you going to use the card for? simple 2d work, compositing, 3d apps, native games, wine games, dual-booting to windows, watching videos, watching HD videos, ...?
The best choice of card and driver differs depending on your usage.


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